Also Occitan: https://fr.wiktionary.org/wiki/Carolina#Occitan (Sources: Frédéric Mistral, Lou Tresor dóu Félibrige ou Dictionnaire provençal-français embrassant les divers dialectes de la langue d’oc moderne, 1879 Josiana Ubaud, Diccionari ortografic, gramatical e morfologic de l’occitan segon los parlars lengadocians, Trabucaire, 2011)
― Anonymous User 6/25/2019
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More than 99.9 percent of people with the first name Carolina are female. Also Catalan and Galician.
― Anonymous User 6/6/2017
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Carolina is also Romanian, though it's not as common. I know a Romanian Carolina.
Source: "Vornamen in der Schweiz. Prénoms en Suisse. I nomi in Svizzera. Prenoms in Svizra" (1993) published by the Association of Swiss registrars
https://sursassiala.ch/2015/01/15/familienforschung/
https://www.portraitarchiv.ch/portrait?page=90
http://www.annalas.ch/persunas/display/q:Carolina