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Emma Charlotte is a good combo (it makes me think of the Brontës for some reason even though Emma isn't Emily), but I wouldn't like it as a proposed IRL name.
Charlotte Grace is good too.

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If Charlotte is the first name, you can get away with a simple/common middle name like Emma or Grace, but if Charlotte is the middle name you'd need a more interesting first name to avoid it looking like a filler.

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Charlotte Rose
Charlotte Anna
Charlotte Elspeth
Charlotte Ophelia
Charlotte Peony
Charlotte Poppy
Charlotte Viola
Charlotte Marigold
Charlotte Eve
Charlotte May
Charlotte Sylvie
Charlotte Pascale
Charlotte Vivienne

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Anna Charlotte
Lily Charlotte
Peony Charlotte
Elizabeth Charlotte
Rosalind Charlotte
Eleanor Charlotte
Viola Charlotte
Sylvia Charlotte
Esther Charlotte
Maia Charlotte
Olwen Charlotte
Aria Charlotte