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I don't mind it. I know a boy named Laine Quinn (not Layne, I know, but still). Quinn is his last name but I always thought it would make a good combo.
I think it would work best as a MN in your family, for a girl or a boy. For boys I'd give it a simple but obviously masculine fn, since Layne (Lane, Laine, etc.) is unisex and the Layne spelling is probably more common for girls.